Wednesday, July 29, 2015

Tuesday 28 July 2015 - Marco Grilli - Nanoscopic inhomogeneity, intrinsic charge instability, and novel metal-to-superconductor quantum criticality in oxide heterostructures


Marco reviewed a number of experimental results on LAO/STO and argued that they indicat a high degree of inhomogeneity in the superconducting state. He emphasized two key observations:

1. The temperature range where resistance starts deviating from the metallic value -- but without vanishing completely -- is much larger than T_c itself.  This behavior is typical for granular superconducting materials.   

2. The resistance curves exhibit long low-temperature tails which are characteristic for systems exhibiting a percolation transition.

Based on these observation, Marco and collaborators proposed that in the “underdoped” side of the superconducting dome, LAO/STO is in a phase separated state. Here, nanoscale superconducting puddles are embedded in a metallic background. As a consequence, below the percolation threshold there is no long-range phase coherence, which is suggested as an explanation for the experimentally observed pseudogap behavior.

Marco then explained that the phase separated state may originate from an intrinsic mechanism. The charge carriers at the interface (electrons) and the outer surface (holes) arise from electronic reconstruction due to the polarity of the system. If the system forms puddles of higher and lower charge carrier concentration,  then it is electrostatically favorable for the electrons to mirror the hole puddles. Moreover, the hole density determines the depth of the potential well experienced by the electrons, and correspondingly the strength of the spin-orbit coupling. The key result was that such a phase separated state may be energetically favorable over a homogeneous state, as indicated by a negative compressibility.

Marco predicted that within this scenario the superconducting fluctuations exhibit an anomalous dynamical critical exponent. This affects a number of observables and may offer a route to experimentally testing the theory.

Blogged by Karen Michaeli

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